Real-Space Imaging of Surface Carrier Transport in 2D Perovskites
Chinese Academy of SciencesUnderstanding photogenerated carrier transport in 2D perovskites, especially surface states, is challenging with conventional time-resolved techniques. Scientists at KAUST utilized scanning ultrafast electron microscopy (SUEM) with groundbreaking surface sensitivity to disclose carrier diffusion rates of ~30 cm虏/s for n=1, 180 cm虏/s for n=2, and 470 cm虏/s for n=3, which are notably higher than bulk. This highlights the SUEM鈥檚 potential for advancing the understanding of carrier dynamics. Density Functional Theory (DFT) confirms broader carrier transmission channels at the surface, offering key insights for optimizing 2D perovskite optoelectronic devices.